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UV-light-induced hydrogen transfer in guanosine-guanosine aggregates (99 visite)

Hunger K, Buschhaus L, Biemann L, Braun M, Kovalenko S, Improta R, Kleinermanns K

Chemistry (ISSN: 0947-6539, 1521-3765, 1521-3765electronic), 2013 Apr; 19(17): 5425-5431.

Tipo di articolo: Journal Article,

Impact factor: 5.696

Impact factor a 5 anni: 5.608


Parole chiave: Aggregation, Hydrogen Transfer, Nucleosides, Photochemistry, Radicals, Experimental Spectra, Quantum Chemical Calculations, Spectroscopic Detection, Transient Absorption, Uv Visible Spectroscopy, Agglomeration, Biomolecules, Photochemical Reactions, Proton Transfer, Quantum Chemistry, Ultraviolet Visible Spectroscopy, Guanosine, Hexane, N-Hexane, Solvent, Article, Chemical Structure, Hydrogen Bond, Methodology, Ultraviolet Radiation, Hydrogen Bonding, Molecular Structure, Photochemical Processes, Spectrum Analysis,

Url: http://www.scopus.com/inward/record.url?eid=2-s2.0-84876259412&partnerID=40&md5=3cc68e703f2b6390e3d92dff9d9823f4

Aggregates of a lipophilic guanine (G) derivative have been studied in n-hexane by femtosecond-to-microsecond UV-visible broadband transient absorption, stationary infrared and UV-visible spectroscopy and by quantum chemical calculations. We report the first time-resolved spectroscopic detection of hydrogen transfer in GG aggregates, which leads to (G-H)· radicals by means of G+G- charge transfer followed by proton transfer. These radicals show a characteristic electronic spectrum in the range 300550 nm. The calculated superimposed spectrum of the species that result from NH⋯N proton transfer agrees best with the experimental spectrum. Copyright © 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
*** IBB - CNR ***

Institute of Physical Chemistry, Heinrich-Heine-University, 40225 Düsseldorf, Germany

Department of Chemistry, Humboldt University, 12489 Berlin, Germany

Istituto Biostrutture e Bioimmagini, CNR, 80134 Napoli, Italy
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* The role of the Cys2-Cys7 disulfide bridge in the early steps of Islet amyloid polypeptide aggregation: A molecular dynamics study (86 visite)
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* Haptoglobin binding to apolipoprotein A-I prevents damage from hydroxyl radicals on its stimulatory activity of the enzyme lecithin-cholesterol acyl-transferase (81 visite)
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* Molecular dynamics analyses of cross-beta-spine steric zipper models: beta-sheet twisting and aggregation (109 visite)
Esposito L, Pedone C, Vitagliano L
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* Molecular mechanism of the inhibition of cytochrome c aggregation by Phe-Gly (99 visite)
La Rosa C, Milardi D, Amato E, Pappalardo M, Grasso D
Arch Biochem Biophys (ISSN: 0003-9861), 2005 Mar 1; 435(1): 182-189.
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* Interplay of electronic, environmental, and vibrational effects in determining the hyperfine coupling constants of organic free radicals (77 visite)
Improta R, Barone V
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* Solvent polarity and pH effects on the magnetic properties of ionizable nitroxide radicals: A combined computational and experimental study of 2, 2, 5, 5-tetramethyl-3-carboxypyrrolidine and 2, 2, 6, 6-tetramethyl-4-carboxypiperidine nitroxides (65 visite)
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Novel insights on nucleoamino acids: biomolecular recognition and aggregation studies of a thymine-conjugated L-phenyl alanine (32 visite)
Roviello G
Amino Acids, N/D; N/D: N/D-N/D.
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