Tin(IV) catalyzed D-galacturonic acid anomerization (226 visite)
Dalton T (ISSN: 1477-9226, 1477-9234, 1477-9234electronic), 2008 Feb 7; (5): 596-601.
Tipo di articolo: Journal Article,
Impact factor: 3.58, Impact factor a 5 anni: 3.409
Url: http://www.scopus.com/inward/record.url?eid=2-s2.0-38549175678&partnerID=40&md5=3db2ef887ed56752e0b03829fb72c65c
Parole chiave: Aldehydes, Catalysis, Enthalpy, Ligands, Nucleophiles, Anomerization, Carboxylic Tail, Galacturonic Acid, Mutarotation Rate Profiles, Nucleophilic Attack, Reaction Kinetics, Hexuronic Acid, Tin Derivative, Article, Chemistry, Nuclear Magnetic Resonance Spectroscopy, Stereoisomerism, Tin Compounds,
Affiliazioni:
*** IBB - CNR ***
Dipartimento CICACF, Università di Messina-Salita Sperone, 31-98166 S.Agata-Messina, Italy
Dipartimento di Chimica Inorganica e Analitica, Università di Palermo, Viale delle Scienze Parco D'Orleans II, I-90123 Palermo, Italy
IBB-CNR Catania, via A. Doria 6, 95125-Catania, Italy
Dipartimento CICACF-Universita di Messina-Salita Sperone, 31-98166 S.Agata-Messina, Italy. arotondo@unime.it,
Riferimenti:
Angyal, S.J., (1980) Chem. Soc. Rev., 9, p. 41
Verchere, J.-F., Chapelle, S., Xin, F., Crans, D.C., (1998) Prog. Inorg. Chem., 47, p. 837
Parulli, U., Floriani, C., (1997) Prog. Inorg. Chem., 45, p. 393. , -429
Brett, C.T., Waldron, K.W., (1990) The Physiology and Biochemistry of Plant Cell Wall, Ed., , Unwin Hyman, Chapman & Hall, London
Ramamoorthy, S., Leppard, G.G., (1977) J. Theor. Biol., 66 (3), p. 527
Tang -. H, R., Belton, P.S., Davies, S.C., Hughes, D.L., (2001) Carbohydr. Res., 330 (3), p. 391
Brown, W.H., Foote, C.S., (1998) Organic Chemistry, , Saunders College Publishing, Orlando, Florida, USA, 2nd edn
Angyal, S.J., (1991) Adv. Carbohydr. Chem. Biochem., 49, p. 20
Brønsted, J.N., Guggenheim, E.A., (1927) J. Am. Chem. Soc., 49, p. 2554
Ryu, K.-S., Kim, C., Kim, I., Yoo, S., Choi, B.-S., Park, C., (2004) J. Biol. Chem., 279 (24), p. 25544. , -25548
Sehray, K.J., Benkovic, S.J., (1978) Acc. Chem. Res., 2, p. 136. , -141
Sneyder, G.R., Serianni, A.S., (1991) Carbohydr. Res., 210, p. 21. , -38
Anderson, L., Garver, J.C., Computer Modeling of the Kinetic of Tautomerization (Mutarotation) of aldoses: Implications for the Mechanism of the Process in (1973) Carbohydrates in Solution, Advances in Chemistry, Series, 117, Ed., , R. Gould, American Chemical Society, Washington D.C., p. 20
Bertazzi, N., Bruschetta, G., Casella, G., Pellerito, L., Rotondo, E., Scopelliti, M., (2003) Appl. Organomet. Chem., 17, p. 932. , -939
Ramos, M.L., Caldeira, M.M., Gil, V.M.S., (1997) Carbohydr. Res., 297 (3), p. 191. , -200
Capon, B., (1969) Chem. Rev., 69 (4), p. 407. , -498
Capon, B., Walker, R.B., (1974) J. Chem. Soc., Perkin Trans. 2, p. 1600. , -1610
Swain, C.G., (1950) J. Am. Chem. Soc., 72, p. 4578. , -4583
Swain, C.G., Brown, J.F., (1952) J. Am. Chem. Soc., 74, p. 2534. , -2538
O'Connor, C.J., Odell, A.L., Bailey, A.T., (1983) Aust. J. Chem., 36, p. 279. , -287
Beebe, J.A., Arabshahi, A., Clifton, J.G., Ringe, D., Petsko, G.A., Frey, P.A., (2003) Biochemistry, 42, p. 4414. , -4420
Nowacki, A., Smiatoczova, K., Kasprzykowska, R., Domochowska, B., Wisniewski, A., (2002) Carbohydr. Res., 337, p. 265. , -272
Isbell, H.S., Frush, H.L., Wade, C.W.R., Hunter, C.E., (1969) Carbohydr. Res., 9, p. 163. , -175
Serianni, A.S., Pierce, J., Huang, S.-G., Barker, R., (1982) J. Am. Chem. Soc., 15, p. 4037. , -4044
Ernst, R.R., Bodenhausen, G., Wokaun, A., (1990) Principles of Nuclear Magnetic Resonance, , Oxford Science Publications, Oxford, UK
Zolnai, Z., Juranic, N., Vikic-Topic, D., MacUra, S., (2000) J. Chem. Inf. Comput. Sci., 40, p. 611
Cobas, J.C., Martin-Pastor, M., (2004) EXSY Calc, Version 1.0, ©, , Mestrec, Universidad de Santiago de Compostela, Spain
Sandstrom, J., (1982) Dynamic NMR Spectroscopy, , Academic Press Inc. Ltd, London, pp. 80-81
Budzelaar, P.H.M., (1995) G-NMR, Version 4.0, , Cherwell Scientific Publishing, Palo Alto, CA, USA, ©
Angyal, S. J., (1980) Chem. Soc. Rev., 9, p. 41
Verchere, J. -F., Chapelle, S., Xin, F., Crans, D. C., (1998) Prog. Inorg. Chem., 47, p. 837
Brett, C. T., Waldron, K. W., (1990) The Physiology and Biochemistry of Plant Cell Wall, Ed., , Unwin Hyman, Chapman & Hall, London
Brown, W. H., Foote, C. S., (1998) Organic Chemistry, , Saunders College Publishing, Orlando, Florida, USA, 2nd edn
Angyal, S. J., (1991) Adv. Carbohydr. Chem. Biochem., 49, p. 20
Br nsted, J. N., Guggenheim, E. A., (1927) J. Am. Chem. Soc., 49, p. 2554
Ryu, K. -S., Kim, C., Kim, I., Yoo, S., Choi, B. -S., Park, C., (2004) J. Biol. Chem., 279 (24), p. 25544. , -25548
Sehray, K. J., Benkovic, S. J., (1978) Acc. Chem. Res., 2, p. 136. , -141
Sneyder, G. R., Serianni, A. S., (1991) Carbohydr. Res., 210, p. 21. , -38
Ramos, M. L., Caldeira, M. M., Gil, V. M. S., (1997) Carbohydr. Res., 297 (3), p. 191. , -200
Swain, C. G., (1950) J. Am. Chem. Soc., 72, p. 4578. , -4583
Swain, C. G., Brown, J. F., (1952) J. Am. Chem. Soc., 74, p. 2534. , -2538
O'Connor, C. J., Odell, A. L., Bailey, A. T., (1983) Aust. J. Chem., 36, p. 279. , -287
Beebe, J. A., Arabshahi, A., Clifton, J. G., Ringe, D., Petsko, G. A., Frey, P. A., (2003) Biochemistry, 42, p. 4414. , -4420
Isbell, H. S., Frush, H. L., Wade, C. W. R., Hunter, C. E., (1969) Carbohydr. Res., 9, p. 163. , -175
Serianni, A. S., Pierce, J., Huang, S. -G., Barker, R., (1982) J. Am. Chem. Soc., 15, p. 4037. , -4044
Ernst, R. R., Bodenhausen, G., Wokaun, A., (1990) Principles of Nuclear Magnetic Resonance, , Oxford Science Publications, Oxford, UK
Cobas, J. C., Martin-Pastor, M., (2004) EXSY Calc, Version 1. 0, , , Mestrec, Universidad de Santiago de Compostela, Spain
Budzelaar, P. H. M., (1995) G-NMR, Version 4. 0, , Cherwell Scientific Publishing, Palo Alto, CA, USA,
Dalton T (ISSN: 1477-9226, 1477-9234, 1477-9234electronic), 2008 Feb 7; (5): 596-601.
Tipo di articolo: Journal Article,
Impact factor: 3.58, Impact factor a 5 anni: 3.409
Url: http://www.scopus.com/inward/record.url?eid=2-s2.0-38549175678&partnerID=40&md5=3db2ef887ed56752e0b03829fb72c65c
Parole chiave: Aldehydes, Catalysis, Enthalpy, Ligands, Nucleophiles, Anomerization, Carboxylic Tail, Galacturonic Acid, Mutarotation Rate Profiles, Nucleophilic Attack, Reaction Kinetics, Hexuronic Acid, Tin Derivative, Article, Chemistry, Nuclear Magnetic Resonance Spectroscopy, Stereoisomerism, Tin Compounds,
Affiliazioni:
*** IBB - CNR ***
Dipartimento CICACF, Università di Messina-Salita Sperone, 31-98166 S.Agata-Messina, Italy
Dipartimento di Chimica Inorganica e Analitica, Università di Palermo, Viale delle Scienze Parco D'Orleans II, I-90123 Palermo, Italy
IBB-CNR Catania, via A. Doria 6, 95125-Catania, Italy
Dipartimento CICACF-Universita di Messina-Salita Sperone, 31-98166 S.Agata-Messina, Italy. arotondo@unime.it,
Riferimenti:
Angyal, S.J., (1980) Chem. Soc. Rev., 9, p. 41
Verchere, J.-F., Chapelle, S., Xin, F., Crans, D.C., (1998) Prog. Inorg. Chem., 47, p. 837
Parulli, U., Floriani, C., (1997) Prog. Inorg. Chem., 45, p. 393. , -429
Brett, C.T., Waldron, K.W., (1990) The Physiology and Biochemistry of Plant Cell Wall, Ed., , Unwin Hyman, Chapman & Hall, London
Ramamoorthy, S., Leppard, G.G., (1977) J. Theor. Biol., 66 (3), p. 527
Tang -. H, R., Belton, P.S., Davies, S.C., Hughes, D.L., (2001) Carbohydr. Res., 330 (3), p. 391
Brown, W.H., Foote, C.S., (1998) Organic Chemistry, , Saunders College Publishing, Orlando, Florida, USA, 2nd edn
Angyal, S.J., (1991) Adv. Carbohydr. Chem. Biochem., 49, p. 20
Brønsted, J.N., Guggenheim, E.A., (1927) J. Am. Chem. Soc., 49, p. 2554
Ryu, K.-S., Kim, C., Kim, I., Yoo, S., Choi, B.-S., Park, C., (2004) J. Biol. Chem., 279 (24), p. 25544. , -25548
Sehray, K.J., Benkovic, S.J., (1978) Acc. Chem. Res., 2, p. 136. , -141
Sneyder, G.R., Serianni, A.S., (1991) Carbohydr. Res., 210, p. 21. , -38
Anderson, L., Garver, J.C., Computer Modeling of the Kinetic of Tautomerization (Mutarotation) of aldoses: Implications for the Mechanism of the Process in (1973) Carbohydrates in Solution, Advances in Chemistry, Series, 117, Ed., , R. Gould, American Chemical Society, Washington D.C., p. 20
Bertazzi, N., Bruschetta, G., Casella, G., Pellerito, L., Rotondo, E., Scopelliti, M., (2003) Appl. Organomet. Chem., 17, p. 932. , -939
Ramos, M.L., Caldeira, M.M., Gil, V.M.S., (1997) Carbohydr. Res., 297 (3), p. 191. , -200
Capon, B., (1969) Chem. Rev., 69 (4), p. 407. , -498
Capon, B., Walker, R.B., (1974) J. Chem. Soc., Perkin Trans. 2, p. 1600. , -1610
Swain, C.G., (1950) J. Am. Chem. Soc., 72, p. 4578. , -4583
Swain, C.G., Brown, J.F., (1952) J. Am. Chem. Soc., 74, p. 2534. , -2538
O'Connor, C.J., Odell, A.L., Bailey, A.T., (1983) Aust. J. Chem., 36, p. 279. , -287
Beebe, J.A., Arabshahi, A., Clifton, J.G., Ringe, D., Petsko, G.A., Frey, P.A., (2003) Biochemistry, 42, p. 4414. , -4420
Nowacki, A., Smiatoczova, K., Kasprzykowska, R., Domochowska, B., Wisniewski, A., (2002) Carbohydr. Res., 337, p. 265. , -272
Isbell, H.S., Frush, H.L., Wade, C.W.R., Hunter, C.E., (1969) Carbohydr. Res., 9, p. 163. , -175
Serianni, A.S., Pierce, J., Huang, S.-G., Barker, R., (1982) J. Am. Chem. Soc., 15, p. 4037. , -4044
Ernst, R.R., Bodenhausen, G., Wokaun, A., (1990) Principles of Nuclear Magnetic Resonance, , Oxford Science Publications, Oxford, UK
Zolnai, Z., Juranic, N., Vikic-Topic, D., MacUra, S., (2000) J. Chem. Inf. Comput. Sci., 40, p. 611
Cobas, J.C., Martin-Pastor, M., (2004) EXSY Calc, Version 1.0, ©, , Mestrec, Universidad de Santiago de Compostela, Spain
Sandstrom, J., (1982) Dynamic NMR Spectroscopy, , Academic Press Inc. Ltd, London, pp. 80-81
Budzelaar, P.H.M., (1995) G-NMR, Version 4.0, , Cherwell Scientific Publishing, Palo Alto, CA, USA, ©
Angyal, S. J., (1980) Chem. Soc. Rev., 9, p. 41
Verchere, J. -F., Chapelle, S., Xin, F., Crans, D. C., (1998) Prog. Inorg. Chem., 47, p. 837
Brett, C. T., Waldron, K. W., (1990) The Physiology and Biochemistry of Plant Cell Wall, Ed., , Unwin Hyman, Chapman & Hall, London
Brown, W. H., Foote, C. S., (1998) Organic Chemistry, , Saunders College Publishing, Orlando, Florida, USA, 2nd edn
Angyal, S. J., (1991) Adv. Carbohydr. Chem. Biochem., 49, p. 20
Br nsted, J. N., Guggenheim, E. A., (1927) J. Am. Chem. Soc., 49, p. 2554
Ryu, K. -S., Kim, C., Kim, I., Yoo, S., Choi, B. -S., Park, C., (2004) J. Biol. Chem., 279 (24), p. 25544. , -25548
Sehray, K. J., Benkovic, S. J., (1978) Acc. Chem. Res., 2, p. 136. , -141
Sneyder, G. R., Serianni, A. S., (1991) Carbohydr. Res., 210, p. 21. , -38
Ramos, M. L., Caldeira, M. M., Gil, V. M. S., (1997) Carbohydr. Res., 297 (3), p. 191. , -200
Swain, C. G., (1950) J. Am. Chem. Soc., 72, p. 4578. , -4583
Swain, C. G., Brown, J. F., (1952) J. Am. Chem. Soc., 74, p. 2534. , -2538
O'Connor, C. J., Odell, A. L., Bailey, A. T., (1983) Aust. J. Chem., 36, p. 279. , -287
Beebe, J. A., Arabshahi, A., Clifton, J. G., Ringe, D., Petsko, G. A., Frey, P. A., (2003) Biochemistry, 42, p. 4414. , -4420
Isbell, H. S., Frush, H. L., Wade, C. W. R., Hunter, C. E., (1969) Carbohydr. Res., 9, p. 163. , -175
Serianni, A. S., Pierce, J., Huang, S. -G., Barker, R., (1982) J. Am. Chem. Soc., 15, p. 4037. , -4044
Ernst, R. R., Bodenhausen, G., Wokaun, A., (1990) Principles of Nuclear Magnetic Resonance, , Oxford Science Publications, Oxford, UK
Cobas, J. C., Martin-Pastor, M., (2004) EXSY Calc, Version 1. 0, , , Mestrec, Universidad de Santiago de Compostela, Spain
Budzelaar, P. H. M., (1995) G-NMR, Version 4. 0, , Cherwell Scientific Publishing, Palo Alto, CA, USA,
A comparative kinetic study of anomerization between the four main forms (α/β-pyranosides and α/β-furanosides) of d-galacturonic acid (GalAH2, 1) and tin(iv) complexed d-galacturonate ([Sn(CH 3)2(GalA)(H2O)2], 2) in D 2O, is reported. Important differences are shown by pD vs. mutarotation rate profiles of 1 and 2. Coordination, in fact, causes: i) a spectacular increase of the rate due to kinetic template assistance of the carboxylic tail holding the metal in close proximity to the reactive centre and ii) a change in the dependence of the rate on the pD. Entropic and enthalpic factors contribute to the huge activation energy decrease in 2. Anomerization rates of the complexed ligand are determined by 2D-EXSY cross-peak integration. Analysis of up to twelve direct and reverse rate constants in the pD range 7.0-2.5 evidences ring size memory, and at least one reaction path which bypasses the aldehydo open chain intermediate. Solvent oxygen atom incorporation into the ligand is, at pH 4.5, about ten fold faster when catalyzed by the metal, and proves that the metal-assisted nucleophilic attack of water on the anomeric carbon atom cannot significantly contribute to mutarotation rates that are thousands of times faster. © The Royal Society of Chemistry 2008.
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Doti N, Scognamiglio PL, Madonna S, Scarponi C, Ruvo M, Perretta G, Albanesi C, Marasco D
* New mimetic peptides of the kinase-inhibitory region (KIR) of SOCS1 through focused peptide libraries (294 visite)
Biochemical Journal, 2012 Apr 1; 443: 231-240.
Impact Factor: 4.779
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Sandomenico A, Russo A, Palmieri G, Bergamo P, Gogliettino M, Falcigno L, Ruvo M
* Small peptide inhibitors of acetyl-peptide hydrolase having an uncommon mechanism of inhibition and a stable bent conformation (278 visite)
J Med Chem (ISSN: 0022-2623, 1520-4804, 0022-2623print), 2012 Mar 8; 55(5): 2102-2111.
Impact Factor: 5.614
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Bonaccorso C, Ciadamidaro A, Sgarlata C, Sciotto D, Arena G, Zito V
* Molecular recognition of organic anions by a water-soluble calix[4]arene: Evidence for enthalpy-entropy compensation (146 visite)
Thermochim Acta (ISSN: 0040-6031), 2012 Feb 20; 530: 107-115.
Impact Factor: 1.989
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Truppo E, Supuran CT, Sandomenico A, Vullo D, Innocenti A, Di Fiore A, Alterio V, De Simone G, Monti SM
* Carbonic anhydrase VII is S-glutathionylated without loss of catalytic activity and affinity for sulfonamide inhibitors (235 visite)
Bioorg Med Chem Lett Bioorganic And Medicinal Chemistry Letters (ISSN: 0960-894x), 2012 Feb 15; 22(4): 1560-1564.
Impact Factor: 2.338
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Monti SM, Supuran CT, De Simone G
* Carbonic anhydrase IX as a target for designing novel anticancer drugs (273 visite)
Curr Med Chem (ISSN: 0929-8673, 1875-533x, 1875-533xelectronic), 2012 Feb; 19(6): 821-830.
Impact Factor: 4.07
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Pilla P, Sandomenico A, Malachovsk V, Borriello A, Giordano M, Cutolo A, Ruvo M, Cusano A
* A protein-based biointerfacing route toward label-free immunoassays with long period gratings in transition mode (256 visite)
Biosens Bioelectron (ISSN: 0956-5663, 1873-4235electronic, 0956-5663linking), 2012 Jan 15; 31(1): 486-491.
Impact Factor: 5.437
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Di Fiore A, Maresca A, Supuran CT, De Simone G
* Hydroxamate represents a versatile zinc binding group for the development of new carbonic anhydrase inhibitors (211 visite)
Chem Commun (ISSN: 1359-7345, 1364-548x, 1364-548xelectronic), 2012; 48(70): 8838-8840.
Impact Factor: 6.378
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Castellano I, Merlino A
* γ-glutamyltranspeptidases: Sequence, structure, biochemical properties, and biotechnological applications (183 visite)
Cell Mol Life Sci (ISSN: 1420-682x), 2012; 69(20): 3381-3394.
Impact Factor: 5.615
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Fusco A, Santulli G, Sorriento D, Cipolletta E, Garbi C, Dorn GW, Trimarco B, Feliciello A, Iaccarino G
* Mitochondrial localization unveils a novel role for GRK2 in organelle biogenesis (217 visite)
Cell Signal (ISSN: 0898-6568), 2012; 24(2): 468-475.
Impact Factor: 4.304
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Bonaccorso C, Sgarlata C, Grasso G, Zito V, Sciotto D, Arena G
* A gemini guest triggers the self-assembly of a calixarene capsule in water at neutral pH (142 visite)
Chem Commun (ISSN: 1359-7345, 1364-548x, 1364-548xelectronic), 2011; 47(21): 6117-6119.
Impact Factor: 6.169
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Esposito G, Imperato MR, Ieno L, Sorvillo R, Benigno V, Parenti G, Parini R, Vitagliano L, Zagari A, Salvatore F
* Hereditary Fructose Intolerance: Functional Study of Two Novel ALDOB Natural Variants and Characterization of a Partial Gene Deletion (235 visite)
Hum Mutat (ISSN: 1059-7794, 1098-1004, 1098-1004electronic), 2010 Dec; 31(12): 1294-1303.
Impact Factor: 5.956
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Merlino A, Russo Krauss I, Castellano I, De Vendittis E, Rossi B, Conte M, Vergara A, Sica F
* Structure and flexibility in cold-adapted iron superoxide dismutases: The case of the enzyme isolated from Pseudoalteromonas haloplanktis (271 visite)
J Struct Biol (ISSN: 1047-8477), 2010 Dec; 172(3): 343-352.
Impact Factor: 3.5
Dettagli Esporta in BibTeX Esporta in EndNote
Pedone E, Limauro D, D'Ambrosio K, De Simone G, Bartolucci S
* Multiple catalytically active thioredoxin folds: a winning strategy for many functions (296 visite)
Cell Mol Life Sci Cellular And Molecular Life Sciences (ISSN: 1420-682x), 2010 Nov; 67(22): 3797-3814.
Impact Factor: 7.047
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Limauro D, D'Ambrosio K, Langella E, De Simone G, Galdi I, Pedone C, Pedone E, Bartolucci S
* Exploring the catalytic mechanism of the first dimeric Bcp: Functional, structural and docking analyses of Bcp4 from Sulfolobus solfataricus (184 visite)
Biochimie (ISSN: 1638-6183, 0300-9084, 1638-6183electronic), 2010 Oct; 92(10): 1435-1444.
Impact Factor: 3.787
Dettagli Esporta in BibTeX Esporta in EndNote
Castellano I, Merlino A, Rossi M, La Cara F
* Biochemical and structural properties of gamma-glutamyl transpeptidase from Geobacillus thermodenitrificans: An enzyme specialized in hydrolase activity (302 visite)
Biochimie (ISSN: 0300-9084, 1638-6183, 1638-6183electronic), 2010 May; 92(5): 464-474.
Impact Factor: 3.787
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Pedone E, Limauro D, Bartolucci S
* The Machinery for Oxidative Protein Folding in Thermophiles (vol 10, pg 157, 2008) (170 visite)
Antioxid Redox Signal (ISSN: 1523-0864, 1557-7716, 1523-0864linking), 2010 Jan; 12(1): 157-169.
Impact Factor: 8.209
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Supuran CT, Di Fiore A, Alterio V, Monti SM, De Simone G
* Recent advances in structural studies of the carbonic anhydrase family: The crystal structure of human CA IX and CA XIII (244 visite)
Curr Pharm Des Current Pharmaceutical Design (ISSN: 1381-6128, 1873-4286), 2010; 16(29): 3246-3254.
Impact Factor: 4.774
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Faiella M, Andreozzi C, de Rosales RT, Pavone V, Maglio O, Nastri F, DeGrado WF, Lombardi A
* An artificial di-iron oxo-protein with phenol oxidase activity (176 visite)
Nat Chem Biol (ISSN: 1552-4450), 2009 Dec; 5(12): 882-884.
Impact Factor: 16.058
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Farina AR, Tacconelli A, Cappabianca L, Cea G, Panella S, Chioda A, Romanelli A, Pedone C, Gulino A, Mackay AR
* The alternative TrkAIII splice variant targets the centrosome and promotes genetic instability (242 visite)
Mol Cell Biol (ISSN: 1098-5549, 0270-7306), 2009 Sep 1; 29(17): 4812-4830.
Impact Factor: 6.057
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Speranza A, Ortosecco G, Castaldi E, Nardelli A, Pace L, Salvatore M
* Fully automated synthesis procedure of 4-[18F]fluorobenzaldehyde by commercial synthesizer: amino-oxi peptide labelling prosthetic group (238 visite)
Applied Radiation And Isotopes (ISSN: 1872-9800, 0969-8043, 0969-8043linking), 2009 Sep; 67(9): 1664-1669.
Impact Factor: 1.094
Dettagli Esporta in BibTeX Esporta in EndNote
D'Ambrosio K, Limauro D, Pedone E, Galdi I, Pedone C, Bartolucci S, De Simone G
* Insights into the catalytic mechanism of the Bcp family: functional and structural analysis of Bcp1 from Sulfolobus solfataricus (239 visite)
Proteins (ISSN: 1097-0134, 0887-3585, 1097-0134electronic), 2009 Sep; 76(4): 995-1006.
Impact Factor: 3.085
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Ruggiero I, Cantiello P, Lamberti A, Sorrentino A, Martucci NM, Ruggiero A, Arcone R, Vitagliano L, Arcari P, Masullo M
* Biochemical Characterisation Of The D60a Mutant Of The Elongation Factor 1 Alpha From The Archaeon Sulfolobus Solfataricus (180 visite)
Biochimie (ISSN: 0300-9084, 1638-6183, 1638-6183electronic), 2009 Jul; 91(7): 835-842.
Impact Factor: 3.897
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Wekselman I, Davidovich C, Agmon I, Zimmerman E, Rozenberg H, Bashan A, Berisio R, Yonath A
* Ribosome's mode of function: Myths, facts and recent results (218 visite)
J Pept Sci (ISSN: 1075-2617, 1099-1387, 1075-2617print), 2009 Mar; 15(3): 122-130.
Impact Factor: 1.807
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Ruggiero A, Tizzano B, Pedone E, Pedone C, Wilmanns M, Berisio R
* Crystal Structure of the Resuscitation-Promoting Factor (Delta DUF)RpfB from M. tuberculosis (211 visite)
J Mol Biol (ISSN: 0022-2836, 1089-8638, 1089-8638electronic), 2009 Jan 9; 385(1): 153-162.
Impact Factor: 3.871
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Di Fiore A, Monti SM, Hilvo M, Parkkila S, Romano V, Scaloni A, Pedone C, Scozzafava A, Supuran CT, De Simone G
* Crystal structure of human carbonic anhydrase XIII and its complex with the inhibitor acetazolamide (255 visite)
Proteins (ISSN: 1097-0134, 0887-3585, 1097-0134electronic), 2009 Jan; 74(1): 164-175.
Impact Factor: 3.085
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Gioia M, Monaco S, Van Den Steen PE, Sbardella D, Grasso G, Marini S, Overall CM, Opdenakker G, Coletta M
* The Collagen Binding Domain of Gelatinase A Modulates Degradation of Collagen IV by Gelatinase (236 visite)
J Mol Biol (ISSN: 0022-2836, 1089-8638, 1089-8638electronic), 2009; 386(2): 419-434.
Impact Factor: 3.871
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Hilvo M, Baranauskiene L, Salzano AM, Scaloni A, Matulis D, Innocenti A, Scozzafava A, Monti SM, Di Fiore A, De Simone G, Lindfors M, Janis J, Valjakka J, Pastorekova S, Pastorek J, Kulomaa MS, Nordlund HR, Supuran CT, Parkkila S
* Biochemical characterization of CA IX, one of the most active carbonic anhydrase isozymes (274 visite)
Jbc Papers (ISSN: 0021-9258, 1083-351x, 0021-9258linking), 2008 Oct 10; 283(41): 27799-27809.
Impact Factor: 5.52
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Sciacca MFM, Pappalardo M, Milardi D, Grasso DM, La Rosa C
* Calcium-Activated Membrane Interaction Of The Islet Amyloid Polypeptide: Implications In The Pathogenesis Of Type Ii Diabetes Mellitus (363 visite)
Arch Biochem Biophys, 2008 Sep 15; 65(1-2): 291-298.
Impact Factor: 3.043
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Lauceri R, Fasciglione G, D'Urso A, Marini S, Purrello R, Coletta M
* Kinetic investigation of porphyrin interaction with chiral templates reveals unexpected features of the induction and self-propagation mechanism of chiral memory (246 visite)
J Am Chem Soc (ISSN: 0002-7863, 0002-2786, 1520-5126), 2008 Sep 13; 130(32): 10476-10477.
Impact Factor: 8.091
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Grimaldi P, Ruocco MR, Lanzotti MA, Ruggiero A, Ruggiero I, Arcari P, Vitagliano L, Masullo M
* Characterisation of the components of the thioredoxin system in the archaeon Sulfolobus solfataricus (235 visite)
Extremophiles (ISSN: 1431-0651, 1433-4909, 1433-4909electronic), 2008 Jul; 12(4): 553-562.
Impact Factor: 1.782
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Mandrich L, Menchise V, Alterio V, De Simone G, Pedone C, Rossi M, Manco G
* Functional and structural features of the oxyanion hole in a thermophilic esterase from Alicyclobacillus acidocaldarius (250 visite)
Proteins (ISSN: 0887-3585, 1097-0134, 1097-0134electronic), 2008 Jun; 71(4): 1721-1731.
Impact Factor: 3.419
Dettagli Esporta in BibTeX Esporta in EndNote
Di Fiore A, Pedone C, Antel J, Waldeck H, Witte A, Wurl M, Scozzafava A, Supuran CT, De Simone G
* Carbonic anhydrase inhibitors: the X-ray crystal structure of ethoxzolamide complexed to human isoform II reveals the importance of thr200 and gln92 for obtaining tight-binding inhibitors (241 visite)
Bioorg Med Chem Lett (ISSN: 1464-3405, 0960-894x, 1464-3405electronic), 2008 Apr 15; 18(8): 2669-2674.
Impact Factor: 2.531
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Innocenti A, Scozzafava A, Parkkila S, Puccetti L, De Simone G, Supuran CT
* Investigations of the esterase, phosphatase, and sulfatase activities of the cytosolic mammalian carbonic anhydrase isoforms I, II, and XIII with 4-nitrophenyl esters as substrates (234 visite)
Bioorg Med Chem Lett Bioorganic And Medicinal Chemistry Letters (ISSN: 0960-894x), 2008 Apr 1; 18(7): 2267-2271.
Impact Factor: 2.531
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Ruggiero A, Chambery A, Di Maro A, Parente A, Berisio R
* Atomic Resolution (1. 1 Angstrom) Structure Of The Ribosome-Inactivating Protein Pd-L4 From Phytolacca Dioica L. Leaves (241 visite)
Proteins (ISSN: 0887-3585, 1097-0134, 1097-0134electronic), 2008 Apr; 71(1): 8-15.
Impact Factor: 3.419
Dettagli Esporta in BibTeX Esporta in EndNote
Pedone E, Limauro D, Bartolucci S
* The machinery for oxidative protein folding in thermophiles (192 visite)
Antioxid Redox Signal (ISSN: 1523-0864, 1557-7716, 1523-0864linking), 2008 Jan; 10(1): 157-169.
Impact Factor: 6.19
Dettagli Esporta in BibTeX Esporta in EndNote
Hilvo M, Innocenti A, Monti SM, De Simone G, Supuran CT, Parkkila S
* Recent advances in research on the most novel carbonic anhydrases, CA XIII and XV (202 visite)
Curr Pharm Des Current Pharmaceutical Design (ISSN: 1381-6128, 1873-4286), 2008; 14(7): 672-678.
Impact Factor: 4.399
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Gomez-monterrey Isabel M, Campiglia P, Bertamino A, Aquino C, Mazzoni O, Diurno Maria V, Iacovino R, Saviano M, Sala M, Novellino E, Grieco P
* Synthesis of Novel Indole-Based Ring Systems by Acid-Catalysed Condensation from α-Amino Aldehydes and L-Trp-OMe (138 visite)
Eur J Org Chem (ISSN: 1099-0690), 2008; 2008(11): 1983-1992.
Impact Factor: 0
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Gomez-monterrey IM, Campiglia P, Bertamino A, Aquino C, Mazzoni O, Diurno MV, Iacovino R, Saviano M, Sala M, Novellino E, Grieco P
* Synthesis Of Novel Indole-Based Ring Systems By Acid-Catalyzed Condensation From A-Amino Aldehydes And L-Trp-Ome (168 visite)
European Journal Of Organic Chemistry (ISSN: 1434-193x), 2008; 11: 1983-1992.
Impact Factor: 3.016
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Papa S, Monti SM, Vitale RM, Bubici C, Jayawardena S, Alvarez K, De Smaele E, Dathan N, Pedone C, Ruvo M, Franzoso G
* Insights Into The Structural Basis Of The Gadd45beta-Mediated Inactivation Of The Jnk Kinase, Mkk7/Jnkk2 (233 visite)
Jbc Papers (ISSN: 0021-9258, 1083-351x, 0021-9258linking), 2007 Jun 29; 282(26): 19029-19041.
Impact Factor: 5.581
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Chambery A, Pisante M, Di Maro A, Di Zazzo E, Ruvo M, Costantini S, Colonna G, Parente A
* Invariant Ser211 is involved in the catalysis of PD-L4, type I RIP from Phytolacca dioica leaves (185 visite)
Proteins (ISSN: 0887-3585, 1097-0134, 1097-0134electronic), 2007 Apr 1; 67(1): 209-218.
Impact Factor: 3.354
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Mai A, Rotili D, Tarantino D, Ornaghi P, Tosi F, Vicidomini C, Sbardella G, Nebbioso A, Miceli M, Altucci L, Filetici P
* Small-molecule inhibitors of histone acetyltransferase activity: Identification and biological properties (252 visite)
J Med Chem (ISSN: 0022-2623, 1520-4804, 0022-2623print), 2006 Nov 16; 49(23): 6897-6907.
Impact Factor: 5.115
Dettagli Esporta in BibTeX Esporta in EndNote
D'Ambrosio K, Pedone E, Langella E, De Simone G, Rossi M, Pedone C, Bartolucci S
* A novel member of the protein disulfide oxidoreductase family from Aeropyrum pernix K1: Structure, function and electrostatics (201 visite)
J Mol Biol (ISSN: 0022-2836, 1089-8638, 1089-8638electronic), 2006 Sep 29; 362(4): 743-752.
Impact Factor: 4.89
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Cappiello M, Alterio V, Amodeo P, Del Corso A, Scaloni A, Pedone C, Moschini R, De Donatis GM, De Simone G, Mura U
* A new spot test for sulfhydryl-containing compounds (251 visite)
Anal Biochem, 2006 Mar 14; 79(1-2): 610-611.
Impact Factor: 2.305
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Cappiello M, Alterio V, Amodeo P, Del Corso A, Scaloni A, Pedone C, Moschini R, De Donatis GM, De Simone G, Mura U
* Metal ion substitution in the catalytic site greatly affects the binding of sulfhydryl-containing compounds to leucyl aminopeptidase (269 visite)
Biochemistry (ISSN: 0006-2960, 1520-4995, 1520-4995electronic), 2006 Mar 14; 45(10): 3226-3234.
Impact Factor: 3.633
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D'Ambrosio K, Pailot A, Talfournier F, Didierjean C, Benedetti E, Aubry A, Branlant G, Corbier C
* The first crystal structure of a thioacylenzyme intermediate in the ALDH family: New coenzyme conformation and relevance to catalysis (206 visite)
Biochemistry (ISSN: 0006-2960, 1520-4995, 1520-4995electronic), 2006 Mar 7; 45(9): 2978-2986.
Impact Factor: 3.633
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Limauro D, Pedone E, Pirone L, Bartolucci S
* Identification and characterization of 1-Cys peroxiredoxin from Sulfolobus solfataricus and its involvement in the response to oxidative stress (173 visite)
Febs Journal (ISSN: 1742-464x), 2006 Feb; 273(4): 721-731.
Impact Factor: 3.033
Dettagli Esporta in BibTeX Esporta in EndNote
Arena G, Casnati A, Contino A, Magrì A, Sansone F, Sciotto D, Ungaro R
* Inclusion of naturally occurring amino acids in water soluble calix[4]arenes: A microcalorimetric and 1H NMR investigation supported by molecular modeling (241 visite)
Org Biomol Chem (ISSN: 1477-0520, 1477-0539, 1477-0539electronic), 2006 Jan 21; 4(2): 243-249.
Impact Factor: 2.874
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Zielenkiewicz W, Swierzewski R, Attanasio F, Rialdi G
* Thermochemical, volumetric and spectroscopic properties of lysozyme-poly(ethylene) glycol system (146 visite)
Journal Of Thermal Analysis And Calorimetry (ISSN: 1388-6150), 2006; 83(3): 587-595.
Impact Factor: 1.438
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Grasso G, D'Agata R, Rizzarelli E, Spoto G, D'Andrea LD, Pedone C, Picardi A, Romanelli A, Fragai M, Yeo KJ
* Activity of anchored human matrix metalloproteinase-1 catalytic domain on Au(111) surfaces monitored by ESI-MS (259 visite)
J Mass Spectrom (ISSN: 1076-5174, 1096-9888), 2005 Dec; 40(12): 1565-1571.
Impact Factor: 3.574
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Merlino A, Mazzarella L, Carannante A, Di Fiore A, Di Donato A, Notomista E, Sica F
* The importance of dynamic effects on the enzyme activity: X-ray structure and molecular dynamics of onconase mutants (271 visite)
Jbc Papers (ISSN: 0021-9258, 1083-351x, 0021-9258linking), 2005 May 6; 280(18): 17953-17960.
Impact Factor: 5.854
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Arena G, Bonomo RP, Contino A, Sgarlata C, Spoto G, Tabbì G
* Influence of the coordination geometry on the physicochemical properties of a copper(II) complex with a tailor-made calixarene-based ligand bearing dipyridyl pendants. An ESR, UV-Vis and CV study (209 visite)
Dalton T (ISSN: 1477-9226, 1477-9234, 1477-9234electronic), 2004 Oct 21; (20): 3205-3211.
Impact Factor: 2.926
Dettagli Esporta in BibTeX Esporta in EndNote
Agmon I, Amit M, Auerbach T, Bashan A, Baram D, Bartels H, Berisio R, Greenberg I, Harms J, Hansen HAS, Kessler M, Pyetan E, Schluenzen F, Sittner A, Yonath A, Zarivach R
* Ribosomal crystallography: A flexible nucleotide anchoring tRNA translocation, facilitates peptide-bond formation, chirality discrimination and antibiotics synergism (161 visite)
Febs Lett (ISSN: 0014-5793, 0014-5793print, 1873-3468electronic), 2004 Jun 1; 567(1): 20-26.
Impact Factor: 3.843
Dettagli Esporta in BibTeX Esporta in EndNote
De Simone G, Mandrich L, Menchise V, Giordano V, Febbraio F, Rossi M, Pedone C, Manco G
* A substrate-induced switch in the reaction mechanism of a thermophilic esterase - Kinetic evidences and structural basis (249 visite)
Jbc Papers (ISSN: 0021-9258, 1083-351x, 0021-9258linking), 2004 Feb 20; 279(8): 6815-6823.
Impact Factor: 6.355
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Caridi A, Cufari A, Lovino R, Palumbo R, Tedesco I
* Influence of Yeast on Polyphenol Composition of Wine (142 visite)
Food Technol Biotechnol (ISSN: 1330-9862), 2004 Jan; 42(1): 37-40.
Impact Factor: 0.475
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Zarivach R, Bashan A, Berisio R, Harms J, Auerbach T, Schluenzen F, Bartels H, Baram D, Pyetan E, Sittner A, Amit M, Hansen HAS, Kessler M, Liebe C, Wolff A, Agmon I, Yonath A
* Functional aspects of ribosomal architecture: Symmetry, chirality and regulation (224 visite)
J Phys Org Chem (ISSN: 0894-3230), 2004; 17(11): 901-912.
Impact Factor: 1.211
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Cimino P, Improta R, Bifulco G, Riccio R, Gomez-paloma L, Barone V
* Nucleophilic Cyclopropane Ring Opening in Duocarmycin SA Derivatives by Methanol under Acid Conditions: A Quantum Mechanical Study in the Gas-Phase and in Solution (276 visite)
J Org Chem (ISSN: 0022-3263, 0022-3263linking), 2004; 69(8): 2816-2824.
Impact Factor: 3.462
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Esposito L, Bruno I, Sica F, Raia CA, Giordano A, Rossi M, Mazzarella L, Zagari A
* Crystal structure of a ternary complex of the alcohol dehydrogenase from Sulfolobus solfataricus (217 visite)
Biochemistry (ISSN: 0006-2960, 1520-4995, 1520-4995electronic), 2003 Dec 16; 42(49): 14397-14407.
Impact Factor: 3.922
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De Simone G, Menchise V, Omaggio S, Pedone C, Scozzafava A, Supuran CT
* Design of weakly basic thrombin inhibitors incorporating novel P1 binding functions: Molecular and X-ray crystallographic studies (205 visite)
Biochemistry (ISSN: 0006-2960, 1520-4995, 1520-4995electronic), 2003 Sep 5; 42(30): 9013-9021.
Impact Factor: 3.922
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Bashan A, Zarivach R, Schluenzen F, Agmon I, Harms J, Auerbach T, Baram D, Berisio R, Bartels H, Hansen HAS, Fucini P, Wilson D, Peretz M, Kessler M, Yonath A
* Ribosomal crystallography: Peptide bond formation and its inhibition (253 visite)
Biopolymers (ISSN: 0006-3525, 0006-6352, 0006-3525print), 2003 Sep; 70(1): 19-41.
Impact Factor: 2.733
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Esposito L, Bruno I, Sica F, Raia CA, Giordano A, Rossi M, Mazzarella L, Zagari A
* Structural study of a single-point mutant of Sulfolobus solfataricus alcohol dehydrogenase with enhanced activity (187 visite)
Febs Lett (ISSN: 0014-5793, 0014-5793print, 1873-3468electronic), 2003 Mar 27; 539(1-3): 14-18.
Impact Factor: 3.609
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Guzzi R, Milardi D, La Rosa C, Grasso D, Verbeet MP, Canters GW, Sportelli L
* The effect of copper/zinc replacement on the folding free energy of wild type and Cys3Ala/Cys26Ala azurin (186 visite)
Int J Biol Macromol (ISSN: 0141-8130, 0141-8130linking, 1879-0003electronic), 2003 Jan 15; 31(4-5): 163-170.
Impact Factor: 1.427
Dettagli Esporta in BibTeX Esporta in EndNote
Esposito G, Vitagliano L, Santamaria R, Viola A, Zagari A, Salvatore F
* Structural and functional analysis of aldolase B mutants related to hereditary fructose intolerance (198 visite)
Febs Lett (ISSN: 0014-5793, 0014-5793print, 1873-3468electronic), 2002 Nov 6; 531(2): 152-156.
Impact Factor: 3.912
Dettagli Esporta in BibTeX Esporta in EndNote
Formaggio F, Bonchio M, Crisma M, Peggion C, Mezzato S, Polese A, Barazza A, Antonello S, Maran F, Broxterman QB, Kaptein B, Kamphuis J, Vitale RM, Saviano M, Benedetti E, Toniolo C
* Nitroxyl peptides as catalysts of enantioselective oxidations (273 visite)
Chemistry (ISSN: 0947-6539, 1521-3765, 1521-3765electronic), 2002; 8(1): [d]84-93.
Impact Factor: 4.238
Dettagli Esporta in BibTeX Esporta in EndNote
Menchise V, Corbier C, Didierjean C, Saviano M, Benedetti E, Jacquot JP, Aubry A
* Crystal structure of the wild-type and D30A mutant thioredoxin h of Chlamydomonas reinhardtii and implications for the catalytic mechanism (224 visite)
Biochem J (ISSN: 0264-6021, 1470-8728electronic, 0264-6021linking), 2001 Oct 1; 359(1): 65-75.
Impact Factor: 4.326
Dettagli Esporta in BibTeX Esporta in EndNote
Garzillo AM, Colao MC, Buonocore V, Oliva R, Falcigno L, Saviano M, Santoro AM, Zappala R, Bonomo RP, Bianco C, Giardina P, Palmieri G, Sannia G
* Structural and kinetic characterization of native laccases from Pleurotas ostreatus, Rigidoporus lignosus, and Trametes trogii (224 visite)
Journal Of Protein Chemistry (ISSN: 0277-8033), 2001 Apr; 20(3): 191-201.
Impact Factor: 1.021
Dettagli Esporta in BibTeX Esporta in EndNote
Bonomo RP, Cennamo G, Purrello R, Santoro AM, Zappala R
* Comparison Of Three Fungal Laccases From Rigidoporus Lignosus And Pleurotus Ostreatus: Correlation Between Conformation Changes And Catalytic Activity (200 visite)
J Chem Res (ISSN: 0162-0134, 1873-3344, 0162-0134print), 2001 Jan 1; 83(1): 67-75.
Impact Factor: 1.729
Dettagli Esporta in BibTeX Esporta in EndNote
Grasso D, Milardi D, La Rosa C, Rizzarelli E
* DSC study of the interaction of the prion peptide PrP106-126 with artificial membranes (225 visite)
New J Chem (ISSN: 1144-0546), 2001; 25(12): 1543-1548.
Impact Factor: 2.44
Dettagli Esporta in BibTeX Esporta in EndNote
De Simone G, Galdiero S, Manco G, Lang D, Rossi M, Pedone C
A snapshot of a transition state analogue of a novel thermophilic esterase belonging to the subfamily of mammalian hormone-sensitive lipase (237 visite)
J Mol Biol (ISSN: 0022-2836, 1089-8638, 1089-8638electronic), 2000 Nov 10; 303(5): 761-771.
Impact Factor: 5.388
Dettagli Esporta in BibTeX Esporta in EndNote
Martínez JC, Viguera AR, Berisio R, Wilmanns M, Mateo PL, Filimonov VV, Serrano L
Thermodynamic analysis of α-spectrin SH3 and two of its circular permutants with different loop lengths: Discerning the reasons for rapid folding in proteins (217 visite)
Biochemistry (ISSN: 0006-2960, 1520-4995, 1520-4995electronic), 1999 Jan 12; 38(2): 549-559.
Impact Factor: 4.493
Dettagli Esporta in BibTeX Esporta in EndNote
Vitagliano L, Adinolfi S, Riccio A, Sica F, Zagari A, Mazzarella L
Binding of a substrate analog to a domain swapping protein: X-ray structure of the complex of bovine seminal ribonuclease with uridylyl(2 ', 5 ')adenosine (209 visite)
Protein Sci (ISSN: 0961-8368, 1469-896xelectronic), 1998 Sep; 7(8): 1691-1699.
Impact Factor: 4.44
Dettagli Esporta in BibTeX Esporta in EndNote
CAPASSO S, SICA F, MAZZARELLA L, BALBONI G, GUERRINI R, SALVADORI S
ACID CATALYSIS IN THE FORMATION OF DIOXOPIPERAZINES FROM PEPTIDES CONTAINING TETRAHYDROISOQUINOLINE-3-CARBOXYLIC ACID AT POSITION-2 (252 visite)
Int J Pept Protein Res (ISSN: 0367-8377, 0367-8377print), 1995 Jun; 45(6): 567-573.
Impact Factor: 1.255
Dettagli Esporta in BibTeX Esporta in EndNote
Bonomo RP, Conte E, Marchelli R, Santoro AM, Tabbì G
O2 - scavenger properties of copper(II) complexes with diamino-diamide-type ligands (222 visite)
J Chem Res (ISSN: 0162-0134, 1873-3344, 0162-0134print), 1994 Feb 1; 53(2): 127-138.
Impact Factor: 1.342
Dettagli Esporta in BibTeX Esporta in EndNote
Costanzo LL, De Guidi G, Giuffrida S, Rizzarelli E, Vecchio G
Determination of superoxide dismutase-like activity of copper(II) complexes. Relevance of the speciation for the correct interpretation of in vitro O2 - scavenger activity (263 visite)
J Chem Res (ISSN: 0162-0134, 1873-3344, 0162-0134print), 1993 Jun; 50(4): 273-281.
Impact Factor: 1.342
Dettagli Esporta in BibTeX Esporta in EndNote
Romano M, Cerra M, Salvatore M, Onorati A
Effects of ionizing radiations on the activity of valyl tRNA synthetase isolated from rat liver and from Morris hepatoma 7777 (317 visite)
Tumori (ISSN: 0300-8916, 0300-8916print, 0300-8916linking), 1974 Jul; 60(4): 301-306.
Impact Factor: 0.408
Dettagli Esporta in BibTeX Esporta in EndNote
98 Records (95 escludendo Abstract e Conferenze).
Impact factor totale: 383.387 (372.004 escludendo Abstract e Conferenze).
Impact factor a 5 anni totale: 376.862 (361.582 escludendo Abstract e Conferenze).
Impact factor totale: 383.387 (372.004 escludendo Abstract e Conferenze).
Impact factor a 5 anni totale: 376.862 (361.582 escludendo Abstract e Conferenze).
Esporta in BibTeX Esporta in EndNote
Ultima modifica di Marco Comerci in data Thursday 16 July 2015, 11:53:53
226 visite. Ultima visita in data Monday 30 March 2020, 14:21:51
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