Effect of amino substitution on the excited state dynamics of uracil (591 views)
Photochem Photobiol Sci (ISSN: 1474-905x), 2008 Jul; 7(7): 765-768.
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Paper type: Journal Article, Research Support, Non-U. S. Gov'T,
Impact factor: 2.144, 5-year impact factor: 2.448
Url: http://www.scopus.com/inward/record.url?eid=2-s2.0-46449125837&partnerID=40&md5=d45cf650b6821d6b29e602e44cbbb6fd
Keywords: 5 Amino 2, 4 Dihydroxypyrimidine, 5 Aminouracil Derivative, 6 Aminouracil, Pyrimidine Derivative, Anisotropy, Aqueous Solution, Article, Chemical Analysis, Chemical Reaction Kinetics, Fluorescence, Priority Journal, Waveform, Fluorescence Polarization, Time Factors, Water, Analogs, Chemistry,
Affiliations:
*** IBB - CNR ***
Laboratoire Francis Perrin, CEA/DSM/IRAMIS/SPAM - CNRS URA 2453, CEA Saclay, F-91191, Gif-sur-Yvette, France
Eötvös Lorand University Budapest, Department of Physical Chemistry, P.O. Box 32, 1518 Budapest 112, Hungary
Dipartimento di Chimica, Università Federico II, Complesso Universitario Monte S. Angelo, Via Cintia, I, 80126, Napoli, Italy
Istituto Biostrutture e Bioimmagini/CNR, V. Mezzocannone, 6, 80134, Napoli, Italy
E tv s Lorand University Budapest, Department of Physical Chemistry, P. O. Box 32, 1518 Budapest 112, Hungary
References:
Not available.
Photochem Photobiol Sci (ISSN: 1474-905x), 2008 Jul; 7(7): 765-768.
Export to BibTeX Export to EndNote
Paper type: Journal Article, Research Support, Non-U. S. Gov'T,
Impact factor: 2.144, 5-year impact factor: 2.448
Url: http://www.scopus.com/inward/record.url?eid=2-s2.0-46449125837&partnerID=40&md5=d45cf650b6821d6b29e602e44cbbb6fd
Keywords: 5 Amino 2, 4 Dihydroxypyrimidine, 5 Aminouracil Derivative, 6 Aminouracil, Pyrimidine Derivative, Anisotropy, Aqueous Solution, Article, Chemical Analysis, Chemical Reaction Kinetics, Fluorescence, Priority Journal, Waveform, Fluorescence Polarization, Time Factors, Water, Analogs, Chemistry,
Affiliations:
*** IBB - CNR ***
Laboratoire Francis Perrin, CEA/DSM/IRAMIS/SPAM - CNRS URA 2453, CEA Saclay, F-91191, Gif-sur-Yvette, France
Eötvös Lorand University Budapest, Department of Physical Chemistry, P.O. Box 32, 1518 Budapest 112, Hungary
Dipartimento di Chimica, Università Federico II, Complesso Universitario Monte S. Angelo, Via Cintia, I, 80126, Napoli, Italy
Istituto Biostrutture e Bioimmagini/CNR, V. Mezzocannone, 6, 80134, Napoli, Italy
E tv s Lorand University Budapest, Department of Physical Chemistry, P. O. Box 32, 1518 Budapest 112, Hungary
References:
Not available.
Effect of amino substitution on the excited state dynamics of uracil
The excited state deactivation of two amino-substituted uracils, 5-aminouracil (5AU) and 6-aminouracil (6AU) in aqueous solution was studied by femtosecond fluorescence upconversion. The fluorescence of 6AU decays as fast as that of uracil with a unique time constant of about 100 femtoseconds. The fluorescence of 5AU exhibits a more complex behavior, fundamentally different from what we found in any other uracils: the decays are globally slower (up to several picoseconds) and depend strongly on the wavelength. This difference is attributed to the particular character of the amino group, affecting the out-of-plane motion of the 5-substituent which has been shown to be crucial for the ultrafast internal conversion occurring in uracils. Our observations indicate instead the formation of a transient fluorescent state which in turn is deactivated by a different relaxation process specific to the amino group. © The Royal Society of Chemistry and Owner Societies.
The excited state deactivation of two amino-substituted uracils, 5-aminouracil (5AU) and 6-aminouracil (6AU) in aqueous solution was studied by femtosecond fluorescence upconversion. The fluorescence of 6AU decays as fast as that of uracil with a unique time constant of about 100 femtoseconds. The fluorescence of 5AU exhibits a more complex behavior, fundamentally different from what we found in any other uracils: the decays are globally slower (up to several picoseconds) and depend strongly on the wavelength. This difference is attributed to the particular character of the amino group, affecting the out-of-plane motion of the 5-substituent which has been shown to be crucial for the ultrafast internal conversion occurring in uracils. Our observations indicate instead the formation of a transient fluorescent state which in turn is deactivated by a different relaxation process specific to the amino group. © The Royal Society of Chemistry and Owner Societies.
Effect of amino substitution on the excited state dynamics of uracil
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Effect of amino substitution on the excited state dynamics of uracil
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